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国家自然科学基金(40375038)

作品数:2 被引量:13H指数:2
相关作者:白郁华程艳丽李金龙刘兆荣更多>>
相关机构:北京大学更多>>
发文基金:国家自然科学基金国家重点基础研究发展计划更多>>
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不同人为源排放对珠江三角洲地区O3生成贡献的数值模拟被引量:10
2008年
利用改进的二维欧拉空气质量模式对珠江三角洲地区不同类型人为源排放对该区域臭氧生成的贡献进行了模拟研究.结果表明,珠江三角洲区域臭氧生成受VOCs排放控制,流动源排放VOC最多,对臭氧生成的贡献也最大,分别占臭氧最大小时浓度和平均小时浓度的44%和67%;其次是溶剂和油漆挥发的贡献.点源和面源排放VOC较少,但排放NOx量大,二者对臭氧生成影响是负的.控制所有类型人为源排放,珠江三角洲区域臭氧日均浓度和最大浓度将分别减少78%和90%.模拟结果还显示,受气象场和光化学反应共同影响,珠江三角洲南部区域是臭氧浓度高值区.
程艳丽白郁华李金龙刘兆荣
关键词:空气质量模式人为源臭氧贡献率
Modeling of air quality with a modified two-dimensional Eulerian model: A case study in the Pearl River Delta (PRD) region of China被引量:4
2007年
A modified two-dimensional Eulerian air quality model was used to simulate both the gaseous and particulate pollutant concentrations during October 21-24, 2004 in the Pearl River Delta (PRD) region, China. The most significant improvement to the model is the added capability to predict the secondary organic aerosols (SOA) concentrations because of the inclusion of the SOA formation chemistry. The meteorological input data were prepared using the CALMET meteorological model. The concentrations of aerosol-bound species such as NO3^-, NH4^+, SO4^2-, and SOA were calculated in the fine particle size range (〈2.5 μm). The results of the two-dimensional model were compared to the measurements at the ground level during the PRD Intensive Monitoring Campaign (IMC). Overall, there were good agreements between the measured and modeled concentrations of inorganic aerosol components and O3. Both the measured and the modeled results indicated that the maximum hourly O3 concentrations exceeded the China National Air Quality Standard. The predicted 24-h average SOA concentrations were in reasonable agreement with those predicted by the method of minimum OC/EC ratio.
CHENG Yan-li BAI Yu-hua LI Jin-long LIU Zhao-rong
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